Optically Active Charge Traps And Chemical Defects In Semiconducting Nanocrystals Probed By Pulsed Optically Detected Magnetic Resonance (Springer Theses)

Optically Active Charge Traps And Chemical Defects In Semiconducting Nanocrystals Probed By Pulsed Optically Detected Magnetic Resonance (Springer Theses)

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    Colloidal nanocrystals show much promise as an optoelectronics architecture due to facile control over electronic properties afforded by chemical control of size, shape, and heterostructure. Unfortunately, realizing practical devices has been forestalled by the ubiquitous presence of charge "trap" states which compete with band-edge excitons and result in limited device efficiencies. Little is known about the defining characteristics of these traps, making engineered strategies for their removal difficult.

    This thesis outlines pulsed optically detected magnetic resonance as a powerful spectroscopy of the chemical and electronic nature of these deleterious states. Counterintuitive for such heavy atom materials, some trap species possess very long spin coherence lifetimes (up to 1.6 ┬Ás). This quality allows use of the trapped charge's magnetic moment as a local probe of the trap state itself and its local environment. Beyond state characterization, this spectroscopy can demonstrate novel effects in heterostructured nanocrystals, such as spatially-remote readout of spin information and the coherent control of light harvesting yield.

      Author

      Kipp van Schooten

      Binding

      Hardcover

      EAN

      9783319005898

      Edition

      2013

      ISBN

      3319005898

      Label

      Springer

      Manufacturer

      Springer

      NumberOfPages

      90

      ProductGroup

      Book

      ProductTypeName

      ABIS_BOOK

      PublicationDate

      2013-07-17

      Publisher

      Springer

      Studio

      Springer

      Optically Active Charge Traps and Chemical Defects in Semiconducting Nanocrystals Probed by Pulsed Optically Detected Magnetic Resonance (Springer Theses)

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